Another wrinkle:
FIDE recommends that the king's diameter to height ratio is from .4 to .5. Given that, and the assumption that the king's diameter to square size ratio is from .7 to .8. The OP has a wider range - but I am lazier. Using the FIDE recommended range, I'll say the ideal diameter to height ratio is .45 (mean of the range). In the same spirit, the ideal diameter to square ratio is .75.
So, if the king's height is 4" the acceptable FIDE king diameter range is from 1.6" to 2.0". The ideal diameter base is 1.8" which makes the ideal square is 2.4". Actually the diameter range from 1.6 to 2.0 can be computed:
$ python khdratio.py -k 4
diameter: 1.600 - 2.000
ideals: diameter: 1.800 | square: 2.400
dia | minsq | ideal | maxsq
1.600 | 2.000 | 2.133 | 2.286
1.650 | 2.062 | 2.200 | 2.357
1.700 | 2.125 | 2.267 | 2.429
1.750 | 2.188 | 2.333 | 2.500
1.800 | 2.250 | 2.400 | 2.571
1.850 | 2.313 | 2.467 | 2.643
1.900 | 2.375 | 2.533 | 2.714
1.950 | 2.438 | 2.600 | 2.786
2.000 | 2.500 | 2.667 | 2.857
That ideal diameter of 1.8 is very consistent with the 4" Jaques sets.
@loubalch You are truly a gentleman and a scholar!! Amazing work!