Not necessarily. It's like asking "will a first-grader get better at math quicker if he sits in high school math classes".
I'd rather try to keep playing "higher rateds" until my %age of wins hovers around 60% .. .and then keep playing in that field. Once your %age of wins increases above this window, you are evidently getting better and you can justifiably seek out stronger players.
Conversely, if you are losing more than 60% of your games, you are probably playing too high up and need to seek out lower rated opposition.
This sweet 60% spot really ties to your comfort zone ... because nobody does anything unless its fun ... so getting your a## beaten too often takes the fun away .. but winning too often doesn't push/challenge you enough to improve.
Will I improve faster if I play people better than me? Right now I have my match ups set at the deafult, min -200 and max +200. I'm wondering if it would be beneficial to change it to somthing like min +100 max +300.